RESEARCH PAPER
Old and new wetting liquids separation in grain-based pattern micromodel during wetting cycles
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1
Department of Bioenvironmental Systems Engineering, National Taiwan University, No. 1, Sec. 4, Roosevelt Rd., Taipei 106319, Taiwan (R.O.C.)
2
Graduate Institute of Hydrological and Oceanic Sciences, National Central University, No.300, Jhongda Rd., Jhongli City, Taoyuan County 320, Taiwan (R.O.C)
3
Department of Mechanical Engineering, National Central University, No.300, Jhongda Rd., Jhongli City, Taoyuan County 320, Taiwan (R.O.C)
4
Institute of Agrophysics, Polish Academy of Sciences, Doświadczalna 4, 20-290 Lublin, Poland
Final revision date: 2024-09-29
Acceptance date: 2024-10-16
Publication date: 2024-11-08
Corresponding author
Shao-Yiu Hsu
Department of Bioenvironmental Systems Engineering, National Taiwan University, Taiwan
Int. Agrophys. 2024, 38(4): 447-456
HIGHLIGHTS
- Grain-based micromodel reveals interplay between new and old wetting liquids
- Grain-based micromodel demonstracts the role of wetting films
- Liquid film on grains crucial for old liquid entrapment
- Films provide connection between new and old liquids
- Weak film development enhances the separation of new and old liquids
KEYWORDS
TOPICS
ABSTRACT
In soils, old (residual) water can persist despite new (invading) water infiltration, potentially due to trapped air bubbles isolating old water pockets. However, the mechanisms behind air bubble formation and liquid separation remain unclear. This study aims to investigate the interaction between new and old wetting liquids and the mechanism that traps air bubbles, isolating old water. Using a grain-based pattern micromodel, we examined these processes during a repeated wetting cycle (wetting-drainage-evaporation-wetting). To enhance visualization and evaporation, we used dyed alcohol solutions as the wetting phase, with air as the non-wetting phase. Results indicate that a liquid film on grains plays a crucial role in old liquid entrapment, influenced more by soil wettability than initial liquid content. Strong wettability resulted in significant film development, allowing old and new liquids to connect and potentially mix. In contrast, weak wettability led to air bubble entrapment, isolating old water and preventing its displacement. The findings highlight that soil wettability and wetting film development are key factors in the interaction between new and old wetting liquids.
FUNDING
This work was funded by National Science and Technology Council under grant: NSTC 113-2116-M-002-001- (2024-2025).
CONFLICT OF INTEREST
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
REFERENCES (43)
1.
Berkowitz, B., 2014. Interchange of infiltrating and resident water in partially saturated media. In: Transport and Reactivity of Solutions in Confined Hydrosystems pp. 55-66: Springer.
https://doi.org/10.1007/978-94....
3.
Bodas, D., Khan-Malek, C., 2006. Formation of more stable hydrophilic surfaces of PDMS by plasma and chemical treatments. Microelectron Eng. 83(4), 1277-1279.
https://doi.org/10.1016/j.mee.....
4.
Brooks, J.R., Barnard, H.R., Coulombe, R., McDonnell, J.J., 2010. Ecohydrologic separation of water between trees and streams in a Mediterranean climate. Nat. Geosci. 3(2), 100-104.
https://doi.org/10.1038/ngeo72....
5.
Chaudhury, M.K., Whitesides, G.M., 1991. Direct measurement of interfacial interactions between semispherical lenses and flat sheets of poly (dimethylsiloxane) and their chemical derivatives. Langmuir 7(5), 1013-1025.
https://doi.org/10.1021/la0005....
6.
Chaudhury, M.K., Whitesides, G.M., 1992. Correlation between surface free energy and surface constitution. Science 255(5049), 1230-1232.
https://doi.org/10.1126/scienc....
7.
Concus, P., Finn, R., 1969. On the behavior of a capillary surface in a wedge. Proc. National Academy of Sciences of the United States of America 63(2), 292.
https://doi.org/10.1073/pnas.6....
9.
Dekker, L.W., Oostindie, K., Ritsema, C.J., 2005. Exponential increase of publications related to soil water repellency. Soil Res. 43(3), 403-441.
https://doi.org/10.1071/SR0500....
10.
Dekker, L.W., Ritsema, C.J., 2000. Wetting patterns and moisture variability in water repellent Dutch soils. J. Hydrol. 231-232, 148-164.
https://doi.org/10.1016/S0022-....
11.
Doerr, S.H., Thomas, A.D., 2000. The role of soil moisture in controlling water repellency: new evidence from forest soils in Portugal. J. Hydrol. 231-232, 134-147.
https://doi.org/10.1016/S0022-....
12.
Fan, L.T., Yuan, X., Zhou, C.X., Zeng, A.W., Yu, K.T., Kalbassi, M., et al., 2011. Contact Angle of Ethanol and n-Propanol Aqueous Solutions on Metal Surfaces. Chem. Eng. Technol. 34.
https://doi.org/10.1002/ceat.2....
13.
Finkenbiner, C.E., Good, S.P., Renée Brooks, J., Allen, S.T., Sasidharan, S., 2022. The extent to which soil hydraulics can explain ecohydrological separation. Nat Commun. 13(1), 6492.
https://doi.org/10.1038/s41467....
14.
Geistlinger, H., Ding, Y., Apelt, B., Schlüter, S., Küchler, M., Reuter, D., et al., 2019. Evaporation study based on micromodel experiments: Comparison of Theory and Experiment. Water Resour Res. 55(8), 6653-6672.
https://doi.org/10.1029/2018WR....
15.
Gouet-Kaplan, M., Berkowitz, B., 2011. Measurements of interactions between resident and infiltrating water in a lattice micromodel. Vadose Zone J. 10(2), 624-633.
http://dx.doi.org/10.2136/vzj2....
16.
Gouet-Kaplan, M., Tartakovsky, A., Berkowitz, B., 2009. Simulation of the interplay between resident and infiltrating water in partially saturated porous media. Water Resour Res. 45(5), n/a-n/a.
http://dx.doi.org/10.1029/2008....
17.
Hsu, S.-Y., Zhang, Z.-Y., Tsao, C.-W., 2017. Thermoplastic micromodel investigation of two-phase flows in a fractured porous medium. Micromachines 8(2), 38.
https://www.mdpi.com/2072-666X....
18.
Huang, Q.Z., Huang, J.C., Tsao, C.W., Hsu, S.Y., 2023. Pore doublet micromodel experiments of evaporation influence on pre-event water entrapment and pre-event and event water interaction. Adv. Water Resour. 177.
https://doi.org/10.1016/j.advw....
20.
Kirchner, J.W., Feng, X., Neal, C., 2000. Fractal stream chemistry and its implications for contaminant transport in catchments. Nature 403(6769), 524-527.
https://doi.org/10.1038/350005....
21.
Lake, L.W., 1989. Enhanced Oil Recovery, Prentice Hall, Englewood Cliffs, New Jersey, USA.
23.
Lehmann, P., Assouline, S., Or, D., 2008. Characteristic lengths affecting evaporative drying of porous media. Phys. Rev. E. 77(5), 056309.
https://link.aps.org/doi/10.11....
24.
Liu, Y., Jeng, D.-S., 2019. Pore structure of grain-size fractal granular material. Materials 12(13), 2053.
25.
Ma’shum, M., Farmer, V., 1985. Origin and assessment of water repellency of a sandy South Australian soil. Soil Res. 23(4), 623-626.
26.
Mata, A., Fleischman, A.J., Roy, S., 2005. Characterization of polydimethylsiloxane (PDMS) properties for biomedical micro/nanosystems. Biomed Microdevices 7(4), 281-293.
27.
Oerter, E.J., Bowen, G., 2017. In situ monitoring of H and O stable isotopes in soil water reveals ecohydrologic dynamics in managed soil systems. Ecohydrology 10(4), e1841.
https://doi.org/10.1002/eco.18....
28.
Radolinski, J., Pangle, L., Klaus, J., Stewart, R.D., 2021. Testing the ‘two water worlds’ hypothesis under variable preferential flow conditions. Hydrol Process. 35(6), e14252.
https://doi.org/10.1002/hyp.14....
29.
Ritsema, C.J., Dekker, L.W., 2012. Soil water repellency: Occurrence, consequences, and amelioration. Elsevier.
30.
Roper, M., Davies, S., Blackwell, P., Hall, D., Bakker, D., Jongepier, R., et al., 2015. Management options for water-repellent soils in Australian dryland agriculture. Soil Res. 53(7), 786-806.
31.
Shao, G., Wu, J., Cai, Z., Wang, W., 2012. Fabrication of elastomeric high-aspect-ratio microstructures using polydime-thylsiloxane (PDMS) double casting technique. Sens. Actuator A-Phys. 178, 230-236.
https://doi.org/10.1016/j.sna.....
32.
Shokri, N., Lehmann, P., Or, D., 2009. Characteristics of evaporation from partially wettable porous media. Water Resour. Res. 45(2).
https://doi.org/10.1029/2008WR....
33.
Shokri, N., Or, D., 2011. What determines drying rates at the onset of diffusion controlled stage‐2 evaporation from porous media? Water Resour Res. 47(9).
34.
Sklash, M., Stewart, M., Pearce, A., 1986. Storm runoff generation in humid headwater catchments: 2. A Case study of hillslope and low‐order stream response. Water Resour. Res. 22(8), 1273-1282.
https://doi.org/10.1029/WR022i....
35.
Smith, W., Crane, M.D., 1930. The Jamin effect in cylindrical tubes. J. Am. Chem. Soc. 52(4), 1345-1349.
36.
Tsao, C.-W., Huang, Q.-Z., You, C.-Y., Hilpert, M., Hsu, S.-Y., Lamorski, K., et al., 2020. The effect of channel aspect ratio on air entrapment during imbibition in soil-on-a-chip micromodels with 2D and 2.5 D pore structures. Lab on Chip.
https://doi.org/10.1039/D0LC01....
37.
Tschapek, M., 1984. Criteria for Determining the hydrophilicity-hydrophobicity of Soils. Zeitschrift für Pflanzenernährung und Bodenkunde, 147(2), 137-149.
https://onlinelibrary.wiley.co....
38.
Turton, D.J., Barnes, D.R., Jr., de Jesus Návar, J., 1995. Old and new water in subsurface flow from a forest soil block. J. Environ. Quality 24, 139-146.
https://doi.org/10.2134/jeq199....
39.
Uchida, T., Tromp-van Meerveld, I., McDonnell, J.J., 2005. The role of lateral pipe flow in hillslope runoff response: an intercomparison of non-linear hillslope response. J. Hydrol. 311(1), 117-133.
https://doi.org/10.1016/j.jhyd....
40.
Valat, B., Jouany, C., Riviere, L.M., 1991. Characterization of the wetting properties of air-dried peats and composts. Soil Sci. 152(2), 100-107.
41.
Vorhauer, N., Wang, Y.J., Kharaghani, A., Tsotsas, E., Prat, M., 2015. Drying with formation of capillary rings in a model porous medium. Transp. Porous Media 110(2), 197-223.
https://doi.org/10.1007/s11242....
42.
Wang, Y.-L., Huang, Q.-Z., Hsu, S.-Y., 2023. The displacement of the resident wetting fluid by the invading wetting fluid in porous media using direct numerical simulation. Water 15(14), 2636.
https://www.mdpi.com/2073-4441....
43.
Yu, Y.-S., Wang, M.-C., Huang, X., 2017. Evaporative deposition of polystyrene microparticles on PDMS surface. Sci. Rep. 7(1), 1-9.
https://www.nature.com/article....